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The total-squared-correlation (\\(TSC\\)) is defined by  \\[ TSC({\\mathcal S}) = \\sum_{i=1}^K\\sum_{j=1}^K | s_is_j^t|^2. \\]  We denote by \\(\\theta(K,L)\\) the minimum of \\(TSC(K<L)\\) over all \\((K,L)\\)-signature sets. A signature set for which the minimum is achieved is called optimal. We have \\(TSC({\\mathcal S})= \\text{trace} ((SS^T)^2)= \\text{trace} ((S^TS)^2)\\), where \\(S\\) is the \\(K\\times L\\) matrix with rows the vector \\(s_i\\). The authors study the question of the existence of optimal signature sets for the following cases when \\(K\\leq L: L\\equiv 1\\pmod{4}\\), \\(K=L\\); \\(L\\equiv 2\\pmod{4}\\), \\(K=L\\) or \\(K=L-1\\). The second case is easy and is settled by Theorem 3.  Theorem 3. If \\(L\\equiv2\\pmod{4}\\) and there exists a Hadamard matrix of order \\(L+2\\), then perfect \\((K,L)\\)-signature sets exist for all \\(K\\leq L\\). For the first case, the authors give various results (Theorems 4--7).  Theorem 4. Let \\(H\\) be a Hadamard matrix of order \\(n\\). Then \\(TSC({\\mathcal S}_H)=(n+1)^3 + n(3n+1) - 4\\sigma(H)\\).  Theorem 5. For \\(K=L\\equiv1\\pmod{4}\\), if Hadamard matrices of order \\(L-1\\) exist, then there exists an \\((L,L)\\)-signature set \\({\\mathcal S}\\) with \\(TSC({\\mathcal S})=L^3+(L-1)(3L-2)-4\\sigma(L-1)\\).  Theorem 6. Let \\({\\mathcal C}\\) be an \\((L,L)\\) code with distance distribution \\(A_0, A_1, \\ldots, A_l\\). Then  \\[ TSC(\\phi({\\mathcal C}))=L\\sum_{i=0}^L A_i(L-2i)^2= L\\sum_{j=0}^{(L-1)/2} \\bigl(A_{\\frac{L-1}{2}-j}+ A_{\\frac{L+1}{2}+j}\\bigr) (2j+1)^2. \\]  In particular, \\(\\phi({\\mathcal C})\\) is perfect if and only if \\(A_i=0\\) for \\(i\\not\\in\\{0,(L-1)/2,(L+1)/2\\}\\).  Theorem 7. Let \\(G=\\{g_1,\\ldots,g_L\\}\\) be an Abelian group of order \\(L\\) and let \\(f:G\\to\\{-1,1\\}\\) be a binary function on \\(G\\). Let \\({\\mathcal S}\\) be the \\((L,L)\\)-signature set  \\[ {\\mathcal S}=\\{{\\mathbf s}_g=(f(g_1+g), f(g_2+g),\\ldots,f(g_L+g))\\mid g\\in G\\}. \\]  Then \\(TSC({\\mathcal S}) = L\\sum_{h\\in G} (C_f(h))^2\\), where \\(C_f(x)=\\sum_{y\\in G} f(x+y)f(x)\\) is the autocorrelation of 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