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The conductor-like screening model for real solvents (COSMO-RS) integral equation will be solved by the shifted Legendre collocation method. This method approximates the unknown function with Legendre polynomials. The merits of this algorithm lie in the fact that, on the one hand, the problem will be reduced to a nonlinear system of algebraic equations. On the other hand, we show that the efficiency and accuracy of the shifted Legendre collocation method for solving these equations are remarkable. Also, this method is using a simple computational manner and its error analysis will be discussed by illustrating some theorems. 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