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Buffeting loading systems of long-span cable-bridge structure are constructed by weighted amplitude wave superposition method. Nonlinear model of cable-bridge coupled vibration control system is established and the corresponding system of state space form is described. In order to reduce buffeting loading influence of the wind-induced vibration for the structure and improve the robust performance of the vibration control, based on semiactive vibration control devices and optimal control approach, a feedforward and feedback optimal vibration controller is designed, and an algorithm is presented for the vibration controller. 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