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The authors continue the study of \\(R\\)-pr. In a previous paper [part II, J. Algebra Appl. 1, No. 2, 201-214 (2002; Zbl 1034.16035)], they defined several preradicals associated to a given preradical. Using these preradicals, they introduced several partitions of \\(R\\)-pr. It were also shown applications that classify rings.   In this paper, they consider several operators acting on \\(R\\)-pr, for instance the pseudocomplement, the annihilator and the totalizer, as well as some relations among them.   A preradical \\(\\sigma\\) is called extreme if \\(\\sigma(ES)=0\\) or \\(\\sigma(ES)=ES\\) for each simple \\(R\\)-module \\(S\\), where \\(ES\\) means the injective hull of \\(S\\) and the collection of all extreme preradicals over \\(R\\) is denoted by \\(R\\)-prex. Then it is shown that \\(R\\) is a left V-ring if and only if \\(R\\)-pr=\\(R\\)-prex. -- Let \\(S\\) and \\(T\\) be simple \\(R\\)-modules. 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