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Special cases lead to the intuition that the possibility of such a general expansion is highly dependent on the density of the set \\(\\Lambda\\). In this paper, we give rigorous results about this relationship. Our approach provides an elementary proof of a result of Rieffel as well as an extension of work of Landau. Our final result states that if \\({\\mathcal S}_{\\Lambda, \\varphi}\\) is a Riesz basis for \\(L^2\\), then the asymptotic density of \\(\\Lambda\\) is exactly one.''   In addition, it should be mentioned that the main auxiliary result of this paper is a simple and powerful ``comparison theorem''. This result is of a quite general nature, and it is intrinsically interesting. In a recent paper [\\textit{K. Gr\u00f6chening} and \\textit{H. Razafinjatovo}, ``On Landau's necessary density for sampling and interpolation of band-limited functions'', J. Lond. Math. Soc. (to appear)], it is shown how this comparison principle yields certain celebrated results of Henry Landau. Roughly speaking, this principle, which is proved by elementary operator theory, says that a set of points in phase space corresponding to a frame of coherent states is uniformly at least as thick as one corresponding to a Riesz basis of coherent states. Other variants can be proved, e.g., one can establish a similar connection between Riesz sequences and bases, and ``phase space'' and ``coherent states'' can, depending on the context, be replaced by other reasonable index sets and families of 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