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Let \\({\\mathfrak H}\\) denote a complex Hilbert space and \\(\\text{Herm}^+ ({\\mathfrak H})\\) the cone of positive definite operators. For a \\(\\text{Herm}^+ ({\\mathfrak H})\\)-valued measure \\(\\mu\\) on \\(\\mathbb{V}^*\\) (endowed with the \\(\\sigma\\)-algebra defined by pointwise evaluations) the Laplace transform is defined as  \\[ {\\mathcal L}(\\mu): \\mathbb{V}\\to \\text{Herm}^+ ({\\mathfrak H}), \\quad x\\mapsto \\int_{\\mathbb{V}^*} e^{\\lambda(x)} d\\mu(\\lambda). \\]  The paper under review is concerned with characterizations of positive operator-valued functions \\(\\varphi\\) on cones \\(S\\subseteq\\mathbb{V}\\) as restrictions of Laplace transforms \\({\\mathcal L} (\\mu)|_S\\). It extends previous investigations, e.g. of \\textit{A. E. Nussbaum} [Duke Math. J. 22, 573-582 (1955; Zbl 0066.36001)], \\textit{J. Hoffmann-J\u00f8rgensen} and \\textit{P. Ressel} [Math. Scand. 40, 79-93 (1977; Zbl 0419.46021)], \\textit{E. Dettweiler} [Math. Scand. 45, 311-333 (1979; Zbl 0427.60009)] and \\textit{K. H. Neeb} [Monatsh. Math. 126, 125-160 (1998)]. For the proofs of the main results the reader is referred to the author's doctoral thesis [``Infinite-dimensional complex groups and semigroups: Representations of cones, tubes, and conelike semigroups'', Doctoral dissertation, Darmstadt, University of Technology; in 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