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In papers [Electron. J. Comb. 24, No. 3, Research Paper P3.59, 14 p. (2017; Zbl 1372.52013); Combinatorica 38, No. 1, 115--142 (2018; Zbl 1413.52016)], the first author proved the non-existence of tight chiral \\(n\\)-polytopes for \\(n\\ge 6\\), determined Schl\u00e4fli symbols of tight chiral polyhedra, and classified the so-called atomic chiral polyhedra which could be covered by each tight chiral polyhedron.  The present paper proves the non-existence of tight chiral 5-polytopes, defines atomic chiral polytopes which generalize atomic chiral polyhedra, and gives all atomic chiral 4-polytopes. In the same way, as every tight chiral polytope covers an atomic chiral polytope, all tight chiral 4-polytopes are classified to a great extent.  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