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Using the left-inariant vector fields \\(X_j=\\frac{\\partial}{\\partial x_j}+2y_j\\frac{\\partial}{\\partial t}\\) and \\(Y_j=\\frac{\\partial}{\\partial y_j}-2x_j\\frac{\\partial}{\\partial t}\\) for \\(j=1,\\dots,n\\), one defines the horizontal gradient \\(\\nabla=(X_1,\\dots,X_n,Y_1,\\dots,Y_n)\\) and the sub-Laplacian \\(\\Delta=\\sum_{j=1}^n(X_j^2+Y_j^2)\\). Any vector \\(v=(a_1,\\dots,a_n,b_1,\\dots,b_n)\\in\\mathbb{R}^n\\times\\mathbb{R}^n\\) gives rise to the sub-Laplacian with a drift \\(\\Delta_v=\\Delta+2\\sum_{j=1}^n(a_jX_j+b_jX_j)\\) and to the measure on \\(\\mathbb{H}_n\\) given by \\(\\text{d}\\mu_v(g)=\\psi_v(g)\\text{d}g\\), where \\(\\psi_v(g)=\\exp(\\sum_{j=1}^n(a_jx_j+b_jy_j))\\). Moreover, the Riesz transform of order \\(k=1,2,\\dots\\) is \\(\\mathcal{R}_k=\\nabla^k(-\\Delta_v)^{-k/2}\\). \\par In the above notation, one proves that if \\(k\\) is a positive integer and \\(k\\ne 2\\), then the Riesz transform \\(\\mathcal{R}_k\\) is of weak type \\((1,1)\\) for the measure \\(\\text{d}\\mu_v\\) if and only if \\(k=1\\). Moreover, defining the Littlewood-Paley-Stein operator associated with \\(\\Delta_v\\) by \\(\\mathcal{H}_kf(g)=\\sup_{h>0}\\vert h^{k/2}\\nabla^k \\text{e}^{h\\Delta_v}f(g)\\vert\\) for \\(k=0,1,2,\\dots\\), one proves that the operator \\(\\mathcal{H}_k\\) is of weak type \\((1,1)\\) with respect to the measure \\(\\text{d}\\mu_v\\) if and only if 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