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A Cayley graph on \\(G\\), denoted by \\(\\mathrm{Cay}(G, S)\\), with respect to \\(S\\) is the graph with vertex set \\(G\\) and the edge set \\(\\{\\{g, sg\\} \\mid g \\in G, s \\in S\\}\\). The valency of a Cayley graph \\(\\Gamma = \\mathrm{Cay}(G, S)\\) is \\(|S|\\), and it is connected if and only if \\(G=\\langle S \\rangle\\). There are plenty of papers dealing with the classification of the symmetric Cayley graphs of non-abelian simple groups, and in most cases the classifications are conditional.  In this paper, the authors try to investigate 7-valent symmetric Cayley graphs of finite simple groups. The following theorem is the main result of the paper.  Theorem. Let \\(G\\) be a finite non-abelian simple group and let \\(\\Gamma = \\mathrm{Cay}(G, S)\\) be a symmetric Cayley graph on \\(G\\) with valency 7. For \\(\\alpha \\in V \\Gamma\\), we have either \\(\\Gamma\\) is a normal Cayley graph or one of the following holds:  \\begin{center} \\begin{tabular}{ c c c } & \\(\\Aut\\Gamma\\) & \\(G\\) \\\\ \\hline 1 & \\([2^{18}].\\mathrm{P}\\Omega^+(12, 2)\\) & \\(\\Omega(11, 2)\\) \\\\ 2 & \\((\\mathbb{Z}_7 \\rtimes \\mathbb{Z}_3) \\times A_8\\) & \\(\\mathrm{PSL}(3, 2)\\) \\\\ 3 & \\(((\\mathbb{Z}_7 \\rtimes \\mathbb{Z}_3) \\times A_8) \\rtimes \\mathbb{Z}_2\\) & \\(\\mathrm{PSL}(3, 2)\\) \\\\ 4 & \\(\\mathbb{Z}_2.\\mathrm{PSU}(6, 2)\\) & \\(\\mathrm{PSU}(5, 2)\\) \\\\ 5 & \\(\\mathbb{Z}_2^2.\\mathrm{PSU}(6, 2)\\) & \\(\\mathrm{PSU}(5, 2)\\) \\\\ & \\(\\mathbb{Z}_4 \\times \\mathrm{PSU}(6, 2)\\) & \\\\ 6 & \\(\\mathbb{Z}_2^4 \\times \\mathrm{Sp}(6, 4)\\) & \\(\\mathrm{PSU}(4, 4)\\) \\\\ 7 & \\((\\mathbb{Z}_7 \\rtimes \\mathbb{Z}_3) \\times \\mathrm{AGL}(3, 2)\\) & \\(\\mathrm{PSL}(2, 7)\\) \\\\ \\hline \\end{tabular} \\end{center}  \\begin{itemize} \\item [(1)] \\(\\Aut \\Gamma\\) acts quasiprimitively on \\(V \\Gamma\\) with \\(L = \\mathrm{soc}(\\Aut \\Gamma)\\) being a non-abelian simple group. And \\((L, G) \\cong (P\\Omega^+(12, 2)\\), \\(\\Omega(11, 2))\\), \\((\\mathrm{Sp}(6, 4), \\mathrm{PSU}(4, 4))\\) or \\((A7,A6)\\). \\item [(2)] There exists a maximal intransitive normal subgroup \\(K\\) of \\(A=\\Aut \\Gamma\\) such that the socle of \\(A/K\\), say \\(\\bar{L}\\), is a simple group containing \\(\\bar{G} = GK/K \\cong G\\) properly. Moreover, one of the following holds. \\begin{itemize} \\item [(i)] \\(\\bar{L}\\) is classical simple group. Then \\((\\Aut\\Gamma, G)\\) is one of the seven cases in the table above. \\item [(ii)] Otherwise, up to isomorphism, we have either \\((\\Aut\\Gamma, G) \\cong (\\mathbb{Z}_7 \\times M_{24}, M_{23}),\\) or \\((\\bar{L}, \\bar{G}) \\cong (A_n, A_{n-1})\\) with \\(\\bar{L}_{\\bar{\\alpha}}\\) has a subgroup of index \\(n\\) for \\(\\bar{\\alpha} \\in V\\Gamma_K\\). \\end{itemize} 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