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In a previous paper [\\textit{K.-T. Kim} et al., Mem. Am. Math. Soc. 984, 111 p. (2011; Zbl 1228.32001)], it was shown that any pseudoconvex domain \\(D\\subset \\mathbb H_a\\) with \\({\\mathcal{C}}^{\\omega}\\)-smooth boundary which is not Stein, is biholomorphic to \\(T_a\\times D_0\\) where \\(D_0\\) is a Stein domain in \\(\\mathbb P^{n-1}\\) with \\({\\mathcal{C}}^{\\omega}\\)-smooth boundary and \\(T_a\\) is a one-dimensional torus. The authors achieved this using the technique of variation of domains in a complex Lie group developed in [loc. cit.] applied to \\(\\mathbb H_a\\) as a complex homogeneous space with transformation group \\(GL(n,{\\mathbb{C}})\\).  Now the present authors use this aforementioned technique of variation of domains to characterize the domains with \\({\\mathcal{C}}^{\\omega}\\)-smooth boundary in \\({\\mathcal{H}}_{(a,b)}\\) which are not Stein. Here \\(a, b\\in {\\mathbb{C}}^*\\) with \\(| b| \\geq | a| >1\\) and \\({\\mathcal{H}}_{(a,b)}\\) is the \\textit{Hopf surface with respect to} \\((a,b)\\), i.e. \\({\\mathcal{H}}_{(a,b)}={\\mathbb{C}}^2\\setminus\\{(0,0)\\}/{\\sim}\\), where \\((z,w)\\sim (z',w')\\) if and only if there exists \\(n\\in {\\mathbb{Z}}\\) such that \\(z'=a^n z\\), \\(w'=b^n w\\). Observe that the complex two-dimensional compact manifold \\({\\mathcal{H}}_{(a,b)}\\) is not a complex Lie group. However, \\({\\mathcal{H}}^*_{(a,b)}={\\mathcal{H}}_{(a,b)}\\setminus ({\\mathbf T}_a \\cup {\\mathbf T}_b)\\) is both a complex Lie group and a complex homogeneous space. And this will play a crucial role in the work. As a matter of fact, with the aid of these facts the authors are able to achieve their aforementioned characterization. Here \\({\\mathbf T}_a=T_a\\times \\{0\\}\\), \\({\\mathbf T}_b=\\{0\\}\\times T_b\\) are disjoint compact analytic curves and \\(T_a:={\\mathbb{C}}^*/{\\sim_a}\\) and \\(T_b:={\\mathbb{C}}^*/{\\sim_b}\\) are complex one-dimensional tori. Recall the definition of the equivalence relation \\(\\sim_a\\), say: For \\(z,\\, z'\\in {\\mathbb{C}}^*\\) one defines \\(z\\sim_a z'\\) if and only if there exists \\(n\\in {\\mathbb{Z}}\\) such that \\(z'=a^nz\\) in 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