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The classification problem of isoparametric hypersurfaces in \\(\\mathbb{R}^n\\) and in the hyperbolic space \\(H^n\\) was solved by \\textit{B. Segre} [Atti Accad. Naz. Lincei Rend. (6) 27, 203--207 (1938; Zbl 0019.18403)] and \\textit{E. Cartan} [Ann. Mat. Pura Appl., IV. Ser. 17, 177--191 (1938; Zbl 0020.06505)], respectively. But Cartan's beautiful theory was relatively unnoticed for thirty years, until it was revived in 1970's by \\textit{K. Nomizu}'s survey paper [Bull. Am. Math. Soc. 79, 1184--1188 (1974; Zbl 0275.53003)].   After that \\textit{H. F. M\u00fcnzner} [Math. Ann. 251, 57--71 (1980; Zbl 0417.53030) and Math. Ann. 256, 215--232 (1981; Zbl 0438.53050)] made excellent contributions to the theory of isoparametric hypersurfaces in spheres. He proved that the number \\(g\\) of distinct principal curvatures of an isoparametric hypersurfaces in \\(S^n\\) must be 1,2,3,4 or 6. Cartan classified isoparametric hypersurfaces with \\(g\\leq 3\\). The classification of isoparametric hypersurfaces with \\(g=4\\) or \\(6\\) remained one of the outstanding problems in submanifolds geometry.   M\u00fcnzner showed that for \\(g=6\\), all isoparametric hypersurfaces must have the same multiplicity \\(m\\), and then U. Abresch showed that \\(m\\) must be 1 or 2. In the case \\(m=1\\), \\textit{J. Dorfmeister} and \\textit{E. Neher} proved [Commun. Algebra 13, 2299--2368 (1985; Zbl 0578.53041)] that an isoparametric hypersurface must be homogeneous, but it is not known whether this is true in the case \\(m=2\\).   For \\(g=4\\), there is a much larger and more diverse collection of known examples. After a series of works of many other geometers, \\textit{D. Ferus, H. Karcher} and \\textit{H.-F. M\u00fcnzner} [Math. Z. 177, 479--502 (1981; Zbl 0443.53037)] used representation of Clifford algebra to construct for any integer \\(m_1>0\\) an infinite series of isoparametric hypersurfaces with four principal curvatures having two different multiplicities \\((m_1, m_2)\\), where \\(m_2=k\\delta(m_1)-m_1-1\\), \\(\\delta(m_1)\\) is the integer such that the Clifford algebra \\(C_{m_1-1}\\) has an irreducible representation on \\(\\mathbb{R}^{\\delta(m_1)}\\) and \\(k\\) is any positive integer for which \\(m_2\\) is positive. This kind of isoparametric hypersurfaces are said to be of FKM-type.   The set of FKM-type isoparametric hypersurfaces contains all known examples with \\(g=4\\), except two homogeneous examples with multiplicities \\((m_1,m_2)=(2,2)\\) and \\((4,5)\\). \\textit{S. Stolz} [Invent. Math. 138, 253--279 (1999; Zbl 0944.53035)] that the multiplicities of an isoparametric hypersurface with \\(g=4\\) must be the same as those in the known examples of FKM-type or the two homogeneous exceptions, this adds weight to the conjecture that the known examples are actually the only isoparametric hypersurfaces with \\(g=4\\). In this paper, the authors prove the following  Classification Theorem: Let \\(M\\) be an isoparametric hypersurface of \\(S^n\\) with \\(g=4\\) and multiplicities \\((m_1,m_2)\\) satisfying \\(m_2\\geq 2m_1-1\\). Then \\(M\\) is of FKM-type.  Taken together with the classifications of \\textit{R. Takagi} [J. Differ. Geom. 11, 225--233 (1976; Zbl 0337.53003)] for the case \\(m_1=1\\) and \\textit{H. Ozeki} and \\textit{M. Takeuchi} [T\u00f4hoku Math. J., II. Ser. 27, 515--559 (1975; Zbl 0359.53011)] for \\(m_1=2\\), this theorem handles all possible pairs \\((m_1,m_2)\\) of multiplicities, with the exception of \\((4,5)\\) and 3 pairs of multiplicities, \\((3,4),(6,9),(7,8)\\) corresponding to isoparametric hypersurfaces of FKM-type. For these 4 pairs, the classification problem for isoparametric hypersurfaces remains 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