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This is an extension of the author's previous work [see \\textit{F. Hiai, M. Mizuo} and \\textit{D. Petz}, J. Math. Soc. Japan 54, No. 3, 679--718 (2002; Zbl 1033.46051)]. The paper consists of seven sections. After some preliminaries (Section 1), in Section 2 the notion of the free pressure \\(\\pi\\) is defined and its several properties are proven. In Section 3, its Legendre transform \\(\\eta\\) is studied. Section 4 derives the relations of \\(\\eta\\) with Voiculescu's free entropy \\(\\chi\\) [see \\textit{D. V. Voiculescu}, Invent. Math. 118, No. 3, 411--440 (1994; Zbl 0820.60001)]. It is shown that \\(\\eta\\geq\\chi\\), and they coincide if random variables are free independent. In Section 5, it is shown the equality also occurs, in the case of two variables \\(a\\) and \\(b\\), when \\(a+ib\\) is \\(R\\)-diagonal. In Section 6 a modification \\(\\pi^{(2)}\\) of \\(\\pi\\) is introduced. 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