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Eilenberg} and \\textit{J. C. Moore} [Foundations of relative homological algebra. Providence, RI: American Mathematical Society (AMS) (1965; Zbl 0129.01101)]. An important branch of relative homological algebra was developed by \\textit{M. Auslander} and \\textit{R.-O. Buchweitz} [M\u00e9m. Soc. Math. Fr., Nouv. S\u00e9r. 38, 5--37 (1989; Zbl 0697.13005)]. The concepts and results in this seminal work comprise what is usually known as \\textit{Auslander-Buchweitz approximation theory}.  The main purpose of this paper is to use  Auslander-Buchweitz approximation theory in order to develop, in the general setting provided by an abelian category \\(\\mathcal{C}\\), the theory of left and right Frobenius pairs. The authors introduce the concept of left Frobenius pairs \\((\\mathcal{X}, \\omega)\\) in an abelian category \\(\\mathcal{C}\\) and show how to construct from \\((\\mathcal{X}, \\omega)\\)  a projective exact model structure on \\(\\mathcal{X}^\\vee\\), the subcategory of objects in \\(\\mathcal{C}\\) with finite \\(\\mathcal{X}\\)-resolution dimension, via cotorsion pairs relative to a thick subcategory of \\(\\mathcal{C}\\). Correspondences between these model structures, relative cotorsion pairs, Frobenius pairs, and Auslander-Buchweitz contexts is established. 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