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The first cohomology theory, termed a natural cohomology, is based on an approach that uses the `dual analogue' of the Banach algebra cohomology. The second theory, termed a dual cohomology, is a generalisation of the group cohomology. The author begins by studying multipliers of operator bimodules and then gives the definition and examples of comodules of Hopf \\(C^*\\)-algebras. Next, cohomology theories of Hopf \\(C^*\\)-algebras are developed.NEWLINENEWLINEAmong the main results, it is shown that the dual cohomology of a saturated unital Hopf \\(C^*\\)-algebra \\(S\\) is concentrated in degree zero if and only if \\(S\\) has a counit and \\(S\\otimes S\\) has a codiagonal. This is a Hopf \\(C^*\\)-algebra version of the fact that the Cartier cohomology of a coalgebra \\(C\\) is concentrated in degree zero if and only if \\(C\\) is a coseparable coalgebra (cf. Theorem 3 in [\\textit{Y. Doi}, J. Math. Soc. Japan 33, 31--50 (1981; Zbl 0459.16007)]). A codiagonal in a Hopf \\(C^*\\)-algebra corresponds to a cointegral in a coseparable coalgebra. It is also proven that, for a locally compact group \\(G\\), the vanishing of the first dual cohomology group of the reduced group \\(C^*\\)-algebra \\(C^*_r(G)\\) is equivalent to the amenability of \\(G\\).NEWLINENEWLINENext, the author defines comodules of Hopf von Neumann algebras and constructs cohomology theories in this case. In difference to the Hopf \\(C^*\\)-algebra case, it is shown that there is a natural Hopf von Neumann algebra comodule structure on the dual space of a comodule, and that the dual cohomology with coefficients in a given comodule coincides with the natural cohomology with coefficients in the corresponding dual 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