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The present paper deals with left invariant complex structures on simply connected Lie groups, whose Lie algebra is a tangent or cotangent Lie algebra. As a start, the existence of totally real complex structures is studied, i.e., complex structures \\(J\\) satisfying the constraint \\(J\\mathfrak{h} = V\\). It is shown that, if \\(\\pi\\) is the adjoint representation, this kind of complex structures are associated to non-singular derivations of \\(\\mathfrak{h}\\). Thus, the existence of totally real complex structures on \\(\\mathrm{T}_{\\pi} \\mathfrak{h}\\) implies that \\(\\mathfrak{h}\\) must be nilpotent. Then, the three dimensional case is studied in detail. For the coadjoint representation, the general form of totally real complex structures is given. 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