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paper under review deals with the following problem: characterise the Fano fourfolds \\((X,-K_X)\\) and the surfaces \\(S\\) in \\(X\\) such that \\((X,-K_X)\\) is not slope stable with respect to \\(S\\).NEWLINENEWLINE Slope stability is a stability condition, introduced by \\textit{J. Ross} and \\textit{R. Thomas} [J. Algebr. Geom. 16, No. 2, 201--255 (2007; Zbl 1200.14095)], weaker than \\(K\\)-stability and easier to verify.NEWLINENEWLINE The relevance of this work is well illustrated by a result proved independently by Chen-Donaldson-Sun and Tian stating the equivalence between the existence of K\u00e4hler-Einstein metrics and \\(K\\)-polystability.NEWLINENEWLINE The work under review extends a previous characterisation ([\\textit{J.-M. Hwang} et al., Bull. Lond. Math. Soc. 43, No. 5, 827--839 (2011; Zbl 1244.14028); \\textit{K. Fujita}, Proc. Japan Acad., Ser. A 87, No. 10, 199--202 (2011; Zbl 1236.14040)]) of Fano manifolds \\((X,-K_X)\\) and curves \\(C\\) in \\(X\\) such that \\((X,-K_X)\\) is not slope stable with respect to \\(C\\).NEWLINENEWLINE The proof is based on the observation that if \\((X,-K_X)\\) is not slope stable with respect to \\(S\\), then \\(S\\) is Fano and on the classification of Fano surfaces. 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