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Let \\(\\Omega\\) be a smooth domain in \\(\\mathbb{C}^2\\). The space \\(\\mathbb{C}^2\\) is identified with the set \\(\\mathbb{H}\\) of real quaternions by means of the mapping that associates the pair \\((z_1,z_2) = (x_0 + i x_1, x_2+ix_3)\\) with the quaternion \\(q=z_1+z_2 j\\). Moreover, \\(\\mathcal{R}(\\Omega)\\) denotes the class of (left-)regular (also called hyperholomorphic) functions \\(f=f_1 + f_2 j : \\Omega \\rightarrow \\mathbb{H}\\) in the kernel of the Cauchy-Riemann operator    \\[  \\mathcal{D} = 2 \\left( \\frac{\\partial}{\\partial \\overline{z}_1} + j \\frac{\\partial}{\\partial \\overline{z}_2} \\right) = \\frac{\\partial}{\\partial x_0} + i \\frac{\\partial}{\\partial x_1} + j \\frac{\\partial}{\\partial x_2} -k \\frac{\\partial}{\\partial x_3}, \\]    a variant of the Cauchy-Fueter operator. The space \\(\\mathcal{R}(\\Omega)\\) contains the identity mapping, and every holomorphic mapping \\((f_1,f_2)\\) on \\(\\Omega\\) defines a regular function \\(f=f_1+f_2j\\). The space \\(\\mathcal{R}(\\Omega)\\) exhibits other interesting links with the theory of two complex variables. In particular, it contains the spaces of holomorphic maps with respect to any constant complex structure on \\(\\mathbb{H}\\), not only the standard one.   Let \\(J_1\\), \\(J_2\\) be the complex structures on the tangent bundle \\(T\\mathbb{H} \\cong \\mathbb{H}\\) defined by left multiplication by \\(i\\) and \\(j\\). Let \\(J_1^*\\), \\(J_2^*\\) be the dual structure on the cotangent bundle \\(T^*\\mathbb{H} \\cong \\mathbb{H}\\), and set \\(J_3^* = J_1^* J_2^*\\), which is equivalent to \\(J_3 = - J_1 J_2\\). Let \\(J_p = p_1 J_1 + p_2 J_2 +p_3 J_3\\) be the orthogonal complex structure on \\(\\mathbb{H}\\) defined by a unit imaginary quaternion \\(p = p_1 i +p_2 j +p_3 k\\) in the sphere \\(\\mathbb{S}^2 = \\{ p \\in \\mathbb{H} \\;| \\;p^2=-1 \\}\\). In particular, \\(J_1\\) is the standard complex stucture. Let \\(L_p\\) be the complex structure defined by left multiplication by \\(p\\), let \\(d\\) be the exterior derivative, and let    \\[ \\overline{\\partial}_p = \\frac{1}{2} \\Big( d + p J_p^* \\circ d\\Big) \\]   be the Cauchy-Riemann operator w.r.t. the structures \\(J_p\\) and \\(L_p\\). Moreover, let \\(\\text{Hol}_p(\\Omega,\\mathbb{H}) = \\text{Ker\\,}\\overline{\\partial}_p\\) be the space of holomorphic maps from \\((\\Omega, J_p)\\) to \\((\\mathbb{H},L_p)\\). Then every element of the space \\(\\text{Hol}_p(\\Omega,\\mathbb{H}) \\) is a regular function.  The quaternionic Cayley transformation \\(\\psi(q)= (q+1)(1-q)^{-1}\\) maps the unit ball \\(B\\) diffeomorphically to the right half-space \\(\\mathbb{H}^+ = \\{ q \\in \\mathbb{H} \\;| \\;\\text{Re\\,}(q) >0 \\}\\), where the real part \\(\\text{Re\\,}(q)\\) of a quaternion \\(q = x_0 + i x_1 + j x_2 + k x_3\\) is \\(x_0\\). This Cayley transformation is combined with the directional, \\(p\\)-dependent, Hilbert operators \\(H_p\\) on the unit sphere \\(S = \\partial B\\) of \\(\\mathbb{H}\\) in order to define the three-dimensional directional Hilbert operator \\(H_p^3\\).  A Sobolev-type space \\(W \\frac{1}{\\partial_p} (\\mathbb{H}_0,\\mathbb{H})\\) of \\(\\mathbb{H}\\)-valued functions \\(f\\) of class \\(L^2(\\mathbb{H}_0)\\) is defined in terms of the Cayley transformation. It is proved that for every \\(p \\in \\mathbb{S}^2\\), there exists a \\(\\mathbb{H}\\)-linear bounded Hilbert operator \\(H_p^3\\) on the space \\(W \\frac{1}{\\partial_p} (\\mathbb{H}_0,\\mathbb{H})\\). For every \\(f \\in W \\frac{1}{\\partial_p} (\\mathbb{H}_0,\\mathbb{H})\\), the function \\(R_p^3(f):= f+ H_p^3(f)\\) is the trace of a regular function on \\(\\mathbb{H}^+\\). The functions \\(f\\) in the kernel of \\(H_p^3\\) are in one-to-one correspondence with the \\(CR_p\\)-functions on \\(S\\), the boundary values of holomorphic functions on \\(B\\) with respect to the operator 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