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They play a decisive role in studying several integral operators such as singular integral operators, oscillatory integral operators, maximal functions, and Littlewood-Paley \\(g\\)-functions, among others. In this paper, the authors introduce three rough integral operators in terms of the Mittag-Leffler function. The first operator is the Mittag-Leffler Spherical Maximal Function which is a generalization of the classical Spherical Maximal Function studied by \\textit{E. M. Stein} [Proc. Natl. Acad. Sci. USA 73, 2174--2175 (1976; Zbl 0332.42018)]. They show that the introduced Mittag-Leffler Spherical Maximal Function is a solution of a diffusion equation. The second operator is a Littlewood-Paley \\(g\\)-function type operator. It generalizes the well-known classical Marcinkiewicz integral operator introduced by \\textit{E. M. Stein} [Trans. Am. Math. Soc. 88, 430--466 (1961; Zbl 0105.05104)]. The third operator is the related Discrete Singular Integral Operator with rough kernels considered in [\\textit{D. Fan} et al., Acta Math. Sin., New Ser. 14, No. 2, 235--244 (1998; Zbl 0906.42009); \\textit{J. Duoandikoetxea} and \\textit{J. L. Rubio de Francia}, Invent. Math. 84, 541--561 (1986; Zbl 0568.42012)]. They prove that the three operators are bounded on \\(L^2(\\mathbb{R}^n)\\). However, it is still unknown whether these operators are bounded on \\(L^p(\\mathbb{R}^n)\\) for \\(p\\) is not equal to 2. 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