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Kihara} [J. Homotopy Relat. Struct. 14, No. 1, 51--90 (2019; Zbl 1459.58001); Smooth homotopy of infinite-dimensional \\(C^{\\infty}\\)-manifolds. Providence, RI: American Mathematical Society (AMS) (2023; Zbl 1542.58001)] has succeeded in introducing a Quillen model structure on the category \\(\\mathsf{Diff}\\) of diffeological spaces. This paper, by relating the local systems over \\(K\\left( \\pi,1\\right) \\)-spaces to the model structure of \\(\\mathsf{Diff}\\), proposes a framework of rational homotopy theory for diffeological spaces.\\N\\NThe synopsis of the paper goes as follows.\\N\\N\\begin{itemize}\\N\\item[\\S 2] recalls the definition of a diffeological space, summarizing the equivalence between the category \\(\\mathsf{Set}^{\\Delta^{\\mathrm{op}}}\\)\\ of simplicial sets and [\\textit{H. Kihara}, Smooth homotopy of infinite-dimensional \\(C^{\\infty}\\)-manifolds. Providence, RI: American Mathematical Society (AMS) (2023; Zbl 1542.58001)].\\N\\N\\item[\\S 3] recalls crucial results on \\textit{local systems} [\\textit{A. G\u00f3mez-Tato} et al., Trans. Am. Math. Soc. 352, No. 4, 1493--1525 (2000; Zbl 0939.55010)], establishing the following theorem.\\N\\NTheorem. Let \\(\\mathsf{Ho}\\left( \\mathsf{Diff}_{\\ast}\\right) \\)\\ be the homotopy category of pointed diffeological spaces with its full subcategory \\(\\mathsf{fib}\\mathbb{Q}\\)-\\(\\mathsf{Ho}\\left( \\mathsf{Diff}_{\\ast}\\right) \\)\\ of fiberwise rational connected diffeological spaces of finite type. Then there exists an equivalence of categories\\N\\[\\N\\mathsf{Ho}\\left( \\mathcal{M}_{\\mathbb{Q}}\\right) \\overset{\\simeq }{\\longrightarrow}\\mathsf{fib}\\mathbb{Q}\\text{-}\\mathsf{Ho}\\left( \\mathsf{Diff}_{\\ast}\\right)\\N\\]\\Nwhere \\(\\mathsf{Ho}\\left( \\mathcal{M}_{\\mathbb{Q}}\\right) \\)\\ is the homotopy category of minimal local systems.\\N\\N\\item[\\S 4] gives examples of local systems associated with relative Sullivan algebras, seeing that a relative Sullivan model for a fibration in \\(\\mathsf{Set}^{\\Delta^{\\mathrm{op}}}\\)\\ gives rise to the fiberwise localization of a diffeological space via the realization functor \\(\\left\\vert {}\\right\\vert _{D}\\).\\N\\N\\item[\\S 5] constructs a spectral sequence converging to the singular de Rham cohomology of a diffeological adjunction space with the pullback of relevant local systems. In case of a stratifold obtained by attaching manifolds, the spectral sequence converges to the Souriau-de Rham cohomology algebra of the diffeological space.\\N\\N\\item[Appendix A] establishes that the functor \\(k\\)\\ from the category \\textsf{Stfd}\\ of stratifolds [\\textit{M. Kreck}, Differential algebraic topology. From stratifolds to exotic spheres. Providence, RI: American Mathematical Society (AMS) (2010; Zbl 1420.57002)] to \\(\\mathsf{Diff}\\)\\ [\\textit{T. Aoki} and \\textit{K. Kuribayashi}, Cah. Topol. G\u00e9om. Diff\u00e9r. Cat\u00e9g. 58, No. 2, 131--160 (2017; Zbl 1378.18016)] assigns an adjunction space in \\(\\mathsf{Diff}\\)\\ to a \\(p\\)-stratifold up to smooth homotopy.\\N\\N\\item[Appendix B] constructs a commutative algebraic model for the unreduced suspension of a connected closed manifold, which was used in \\S 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