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Unfortunately, the theory of bilinear integration with respect to a vector measure originating from the work of Bartle cannot be applied due to the singular variational properties of spectral measures. In this work, it is shown how ``decoupled'' bilinear integration may be used to find solutions \\(X\\) of operator equations \\(AX-XB=Y\\) with respect to the spectral measure of \\(A\\) and to apply such representations to the spectral decomposition of block operator matrices. A new proof is given of Peller's characterisation of the space \\(L^1((P\\otimes Q)_{\\mathcal L(\\mathcal H)})\\) of double operator integrable functions for spectral measures \\(P\\), \\(Q\\) acting in a Hilbert space \\(\\mathcal H\\) and applied to the representation of the trace of \\(\\int_{\\Lambda\\times\\Lambda}\\varphi\\) \\(d(PTP)\\) for a trace class operator \\(T\\). The method of double operator integrals due to Birman and Solomyak is used to obtain an elementary proof of the existence of Krein's spectral shift 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