Dynamics and bifurcations on the normally hyperbolic invariant manifold of a periodically driven system with rank-1 saddle
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Publication:2220895
bifurcationnormally hyperbolic invariant manifoldrank-1 saddlestroboscopic maptransition state theory
Dynamical systems with hyperbolic orbits and sets (37D05) Invariant manifold theory for dynamical systems (37D10) Bifurcations of limit cycles and periodic orbits in dynamical systems (37G15) Bifurcation problems for finite-dimensional Hamiltonian and Lagrangian systems (37J20) Simulation of dynamical systems (37M05) Numerical bifurcation problems (65P30)
Abstract: In chemical reactions, trajectories typically turn from reactants to products when crossing a dividing surface close to the normally hyperbolic invariant manifold (NHIM) given by the intersection of the stable and unstable manifolds of a rank-1 saddle. Trajectories started exactly on the NHIM in principle never leave this manifold when propagated forward or backward in time. This still holds for driven systems when the NHIM itself becomes time dependent. We investigate the dynamics on the NHIM for a periodically driven model system with two degrees of freedom by numerically stabilizing the motion. Using Poincar'e surfaces of section we demonstrate the occurrence of structural changes of the dynamics, emph{viz.}, bifurcations of periodic transition state (TS) trajectories when changing the amplitude and frequency of the external driving. In particular, periodic TS trajectories with the same period as the external driving but significantly different parameters---such as mean energy---compared to the ordinary TS trajectory can be created in a saddle-node bifurcation.
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Cited in
(4)- Controlling reaction dynamics in chemical model systems through external driving
- The role of normally hyperbolic invariant manifolds (NHIMS) in the context of the phase space setting for chemical reaction dynamics
- KCC Analysis of the Normal Form of Typical Bifurcations in One-Dimensional Dynamical Systems: Geometrical Invariants of Saddle-Node, Transcritical, and Pitchfork Bifurcations
- Bifurcations of normally hyperbolic invariant manifolds in analytically tractable models and consequences for reaction dynamics
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