A free-boundary problem for concrete carbonation: front nucleation and rigorous justification of the t-law of propagation

DOI10.4171/IFB/299zbMATH Open1276.35127arXiv1102.3452OpenAlexW1556700303MaRDI QIDQ384170FDOQ384170

Authors: Toyohiko Aiki, Adrian Muntean 

Publication date: 26 November 2013

Published in: Interfaces and Free Boundaries (Search for Journal in Brave)

Abstract: We study a one-dimensional free-boundary problem describing the penetration of carbonation fronts (free reaction-triggered interfaces) in concrete. A couple of decades ago, it was observed experimentally that the penetration depth versus time curve (say $s(t)$ vs. $t$) behaves like $s(t)=Csqrtt$ for sufficiently large times $t>0$ (with $C$ a positive constant). Consequently, many fitting arguments solely based on this experimental law were used to predict the large-time behavior of carbonation fronts in real structures, a theoretical justification of the $sqrtt$-law being lacking until now. %This is the place where our paper contributes: The aim of this paper is to fill this gap by justifying rigorously the experimentally guessed asymptotic behavior. We have previously proven the upper bound $s(t)leq{C}^{\prime }sqrtt$ for some constant $C^{\prime }$; now we show the optimality of the rate by proving the right nontrivial lower estimate, i.e. there exists $$ such that $$. Additionally, we obtain weak solutions to the free-boundary problem for the case when the measure of the initial domain vanishes. In this way, our mathematical model is now allowing for the appearance of a moving carbonation front -- a scenario that until was hard to handle from the analysis point of view.

Full work available at URL: https://arxiv.org/abs/1102.3452

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zbMATH Keywords

free-boundary problemlarge-time behaviorintegral estimatesconcrete carbonation

Mathematics Subject Classification ID

PDEs in connection with fluid mechanics (35Q35)

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