From the GKLS equation to the theory of solar and fuel cells

DOI10.1142/S1230161217400078MaRDI QIDQ4595339zbMATH OpenOpenAlexFDO

Authors Robert Alicki

Publication date 30 November 2017

Published in Open Systems & Information Dynamics (Search for Journal in Brave)

Full work available at URL https://arxiv.org/abs/1706.10257

zbMATH Keywords

photovoltaic cellsquantum enginesquantum master equationsquantum thermodynamics

Mathematics Subject Classification ID

Electromagnetic effects in solid mechanics (74F15) Open systems, reduced dynamics, master equations, decoherence (81S22) Statistical thermodynamics (82B30)

Abstract: The mathematically sound theory of quantum open systems, formulated in the 70-ties of XX century and highlighted by the discovery of Gorini-Kossakowski-Lindblad-Sudarshan (GKLS) equation, found a wide range of applications in various branches of physics and chemistry, notably in the field of quantum information and quantum thermodynamics. However, it took 40 years before this formalism has been applied to explain correctly the operation principles of long existing energy transducers like photovoltaic, thermoelectric and fuel cells. This long path is briefly reviewed from the personal author's perspective. Finally, the new, fully quantum model of chemical engine based on GKLS equation and applicable to fuel cells or replicators is outlined. The model illustrates the difficulty with an entirely quantum operational definition of work, comparable to the Problem of Quantum Measurement.

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Cited in

(5)

• On the Floquet analysis of commutative periodic Lindbladians in finite dimension
• Markovian dynamics under weak periodic coupling
• Thermodynamics of Markovian Open Quantum Systems with Application to Lasers
• Thermodynamics and performance optimization of an open quantum engine
• Limitations of the Markovian approximation in the harmonic oscillator

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