Natural break-up and satellite formation regimes of surfactant-laden liquid threads

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Publication:5205735

DOI10.1017/JFM.2019.874zbMATH Open1430.76164arXiv1903.02839OpenAlexW3103851832WikidataQ111199936 ScholiaQ111199936MaRDI QIDQ5205735FDOQ5205735


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Publication date: 16 December 2019

Published in: Journal of Fluid Mechanics (Search for Journal in Brave)

Abstract: We report a numerical analysis of the unforced break-up of free cylindrical threads of viscous Newtonian liquid whose interface is coated with insoluble surfactants, focusing on the formation of satellite droplets. The initial conditions are harmonic disturbances of the cylindrical shape with a small amplitude epsilon, and whose wavelength is the most unstable one deduced from linear stability theory. We demonstrate that, in the limit epsilono0, the problem depends on two dimensionless parameters, namely the Laplace number, , and the elasticity parameter, , where ho, mu and sigma0 are the liquid density, viscosity and initial surface tension, respectively, E is the Gibbs elasticity and is the unperturbed thread radius. A parametric study is presented to quantify the influence of La and on two key quantities: the satellite droplet volume and the mass of surfactant trapped at the satellite's surface just prior to pinch-off, Vsat and Sigmasat, respectively. We identify a weak-elasticity regime, , in which the satellite volume and the associated mass of surfactant obey the scaling law Vsat=Sigmasat=0.0042La1.64 for Lalesssim2. For Lagtrsim10, Vsat and Sigmasat reach a plateau of about 3% and 2.9% respectively, Vsat being in close agreement with previous experiments of low-viscosity threads with clean interfaces. For La<7.5, we reveal the existence of a discontinuous transition at a critical elasticity , with for Lalesssim0.2, such that Vsat and Sigmasat abruptly increase. The jumps experienced by both quantities reach a plateau when Lalesssim0.2, while they decrease monotonically as La increases up to La=7.5, where both become zero.


Full work available at URL: https://arxiv.org/abs/1903.02839




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